Two-photon absorption

Two-photon absorption is theoretically analyzed within the semiclassical formalism of radiation-matter interaction. We consider an ensemble of inhomogeneously broadened three-level atoms subjected to the action of two counterpropagating fields of the same frequency. By concentrating in the limit of large detuning in one-photon transitions, we solve perturbatively the Bloch equations in a non-usual way. In this way we derive an analytical expression for the width of the two-photon resonance that makes evident sub-Doppler two-photon spectroscopy. We also derive an analytical expression for the Stark shift of the two-photon resonance.

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Bibliographic Details
Main Authors: Perez-Arjona,I., Valcárcel,G.J. de, Roldan,Eugenio
Format: Digital revista
Language:English
Published: Sociedad Mexicana de Física 2003
Online Access:http://www.scielo.org.mx/scielo.php?script=sci_arttext&pid=S0035-001X2003000100014
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